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Daniel P. Glavin Jamie E. Elsila Hannah L. McLain Jos C. Aponte Eric T. Parker Jason P. Dworkin Dolores H. Hill Harold C. Connolly Dante S. Lauretta 《Meteoritics & planetary science》2021,56(1):148-173
The abundances, distributions, enantiomeric ratios, and carbon isotopic compositions of amino acids in two fragments of the Aguas Zarcas CM2 type carbonaceous chondrite fall and a fragment of the CM2 Murchison meteorite were determined via liquid chromatography time‐of‐flight mass spectrometry and gas chromatography isotope ratio mass spectrometry. A suite of two‐ to six‐carbon aliphatic primary amino acids was identified in the Aguas Zarcas and Murchison meteorites with abundances ranging from ~0.1 to 158 nmol/g. The high relative abundances of α‐amino acids found in these meteorites are consistent with a Strecker‐cyanohydrin synthesis on these meteorite parent bodies. Amino acid enantiomeric and carbon isotopic measurements in both fragments of the Aguas Zarcas meteorites indicate that both samples experienced some terrestrial protein amino acid contamination after their fall to Earth. In contrast, similar measurements of alanine in Murchison revealed that this common protein amino acid was both racemic (D ≈ L) and heavily enriched in 13C, indicating no measurable terrestrial alanine contamination of this meteorite. Carbon isotope measurements of two rare non‐proteinogenic amino acids in the Aguas Zarcas and Murchison meteorites, α‐aminoisobutyric acid and D‐ and L‐isovaline, also fall well outside the typical terrestrial range, confirming they are extraterrestrial in origin. The detections of non‐terrestrial L‐isovaline excesses of ~10–15% in both the Aguas Zarcas and Murchison meteorites, and non‐terrestrial L‐glutamic acid excesses in Murchison of ~16–40% are consistent with preferential enrichment of circularly polarized light generated L‐amino acid excesses of conglomerate enantiopure crystals during parent body aqueous alteration and provide evidence of an early solar system formation bias toward L‐amino acids prior to the origin of life. 相似文献
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Previous work on identifying opportunities for Pacific Island countries to improve the economic returns from their tuna resources in the Western and Central Pacific Ocean (WCPO) has not generally included articulation of aspirations from Islanders themselves. However, generating such an understanding is increasingly important as these countries assert their positions in regional fisheries policy making. This study analyses the self-identified aspirations of industry and government representatives from six Pacific Island countries and finds a wider diversity of attitudes, strategies and success than is generally recognised. Implications for negotiations in the WCPFC are then discussed. 相似文献
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Matthew G. Hannah 《GeoJournal》2010,75(4):397-406
Ewald’s recent genealogy of constructions of risk in Western societies argues that the 1980s saw an important paradigm shift
to the “precautionary principle”. Critical scholars have taken up this idea as a lens through which to interpret the Bush
administration’s ‘war on terror’. I argue that 11 September 2001 actually brought about qualitative changes to this paradigm.
Bush’s pre-emptive doctrine is driven, and perhaps even more importantly, continually justified to the US population, by what
might be called the “trans-precautionary principle”, a move from “decisionism” to “actionism”, and a new radicalization of
the way fear is produced and managed. Donald Rumsfeld’s famous typology of different articulations of knowledge and ignorance
offers an excellent analytical window onto the connections between ignorance, fear and geopolitical action in this new regime.
In the latter part of the essay, his four modes of knowledge/ignorance are arrayed, for heuristic purposes, in an abstract
spatial grid organized along dimensions of the specificity and possession of knowledge. This allows a ‘mapping’ of some of
the Bush administration’s more controversial strategies in the ‘war on terror’, as a set of different pathways through Rumsfeld
Space. 相似文献
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Aaron S. Burton Hannah McLain Daniel P. Glavin Jamie E. Elsila Jemma Davidson Kelly E. Miller Alexander V. Andronikov Dante Lauretta Jason P. Dworkin 《Meteoritics & planetary science》2015,50(3):470-482
Exogenous delivery of amino acids and other organic molecules to planetary surfaces may have played an important role in the origins of life on Earth and other solar system bodies. Previous studies have revealed the presence of indigenous amino acids in a wide range of carbon‐rich meteorites, with the abundances and structural distributions differing significantly depending on parent body mineralogy and alteration conditions. Here we report on the amino acid abundances of seven type 3–6 CK chondrites and two Rumuruti (R) chondrites. Amino acid measurements were made on hot water extracts from these meteorites by ultrahigh‐performance liquid chromatography with fluorescence detection and time‐of‐flight mass spectrometry. Of the nine meteorites analyzed, four were depleted in amino acids, and one had experienced significant amino acid contamination by terrestrial biology. The remaining four, comprised of two R and two CK chondrites, contained low levels of amino acids that were predominantly the straight chain, amino‐terminal (n‐ω‐amino) acids β‐alanine, and γ‐amino‐n‐butyric acid. This amino acid distribution is similar to what we reported previously for thermally altered ureilites and CV and CO chondrites, and these n‐ω‐amino acids appear to be indigenous to the meteorites and not the result of terrestrial contamination. The amino acids may have been formed by Fischer–Tropsch‐type reactions, although this hypothesis needs further testing. 相似文献
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Regimes are useful tools for characterizing the seasonal behaviour of river flow and other hydroclimatological variables over an annual cycle (hydrological year). This paper develops and tests: (i) a regime classification method to identify spatial and temporal patterns in intraannual hydroclimatological response; and (ii) a novel sensitivity index (SI) to assess river flow regimes' climatic sensitivity. The classification of regime shape (form) and magnitude considers the whole annual cycle rather than isolating a single month or season for analysis, which has been the common approach of previous studies. The classification method is particularly useful for identifying large‐scale patterns in regimes and their between‐year stability, thus providing a context for short‐term, small‐scale process‐based research. The SI provides a means of assessing the often‐complex linkages between climatic drivers and river flow, as it identifies the strength and direction of associations between classifications of climate and river flow regimes. The SI has the potential for application to other problems where relationships between nominal classifications require to be found. These techniques are evaluated by application to a test data set of river flow, air temperature and rainfall time‐series (1974–1999) for a sample of 35 UK river basins. The results support current knowledge about the hydroclimatology of the UK. Although this research does not seek to yield new, detailed physical process understanding, it provides perspective at large spatial and temporal scales upon climate and flow regime patterns and quantifies linkages. Having clearly demonstrated the regime classification and SI to be effective in an environment where the hydroclimatology is relatively well known, there appears to be much to gain from applying these techniques in parts of the world where patterns and associations between climate and hydrology are poorly understood. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
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